作者：Chang Zhang, Peng Xiao,* F. Ni, L.K. Yan, Q.Q. Liu, D. Zhang, J.C. Gu, Wenqin Wang,* and Tao Chen*
关键字：Polypyrrole, Biomass sponge, Low-energy-consumption, Photothermic conversion, Water treatment
论文来源：期刊
具体来源：ACS Sustainable Chem. Eng. 2020, 8, 5328?5337
发表时间：2020年
Converting waste into versatile materials has been considered as an e?ective strategy to tackle environmental issues such as shortages in food, clean water, and energy. Conventional carbonization technology has provided an e?ective approach for constructing photothermal materials for interfacial evaporation or crude oil removal. However, high energy consumption, poor shape retention, and weak mechanical strength have signi?cantly hindered the practical application of conventional carbonization technology. This work discusses how a biomass-derived sponge from discarded pomelo peel (PP) may be used to collect photothermal polypyrrole in a cost-e?ective way with mild reaction. The photothermic sponge which is derived from this process, can then be e?ectively employed to realize solar enhanced water evaporation and heavy crude oil removal. The polypyrrole-functionalized pomelo peel (FPyPP) can be attained by a mild, one-pot wet oxypolymerization method, resulting in over 95% absorption of sunlight and evaporation rates of about 1.22 kg/m2 under the sun. Furthermore, the concentrated heat on the sponge surface can e?ciently reduce the viscosity of heavy crude oil and thereby lead to an e?ective cleanup. This study aims to provide a low-cost, low-energy-consumption, and eco-friendly approach to the acquisition of the multifunctional photothermic sponge by recycling the waste and demonstrating potential applications in tackling clean water generation and polluted water treatment.